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Creators/Authors contains: "Rader, Claire"

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  1. We generate tunable narrowband THz radiation using BNA bonded to sapphire in tandem with a chirp and delay technique. Using a Ti:Sapphire laser, we test the limits of intense THz generation (0.1 to 5 THz). 
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  2. Abstract Large crystal growth and characterization of the optical and terahertz (THz) properties of organic nonlinear optical (NLO) crystal NMBA (4‐Nitro‐4′‐methylbenzylidene aniline) is presented. The reported method of crystal growth consistently produces high‐quality single crystals. The THz generation efficiency and optical properties of NMBA to other THz generation crystals including BNA and MNA are compared. The low THz absorptions that make NMBA an ideal source for THz time‐domain spectroscopy are highlighted. 
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  3. Organic nonlinear optical (NLO) crystals are among the most efficient (>1%) terahertz (THz) radiation generators. However, one of the limitations of using organic NLO crystals is that the unique THz absorptions in each crystal make it difficult to obtain a strong, smooth, and broad emission spectrum. In this work, we combine THz pulses from two complementary crystals, DAST and PNPA, to effectively fill in spectral gaps, creating a smooth spectrum with frequencies out to 5 THz. The combination of pulses also increases the peak-to-peak field strength from 1 MV/cm to 1.9 MV/cm. 
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  4. Nonlinear optical processes with THz frequency light have rarely been measured and characterized. Using 2D THz spectroscopy, we clearly observe THz-optical rectification and THz- second harmonic generation in a variety of materials. 
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  5. We present the optical and THz properties of highly efficient organic nonlinear optical crystals PNPA and MNA. These crystals outperform industry standards in broadband THz generation through optical rectification of IR light pulses. 
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  6. We discover, develop, and test new organic nonlinear optical crystals that produce intense pulses of terahertz radiation through a combination of data mining from Cambridge Structural Database and density functional theory calculations. 
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  7. We discover, develop, and test new organic nonlinear optical crystals that produce intense pulses of terahertz radiation through a combination of data mining from Cambridge Structural Database and density functional theory calculations. 
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